Abstract
When a superconductor is placed close to a non-superconducting metal, it can induce superconducting correlations in the metal 1,2,3,4,5,6,7,8,9,10, known as the ‘proximity effect’11. Such behaviour modifies the density of states (DOS) in the normal metal12,13,14,15 and opens a minigap12,13,16 with an amplitude that can be controlled by changing the phase of the superconducting order parameter12,15. Here, we exploit such behaviour to realize a new type of interferometer, the superconducting quantum interference proximity transistor (SQUIPT), for which the operation relies on the modulation with the magnetic field of the DOS of a proximized metal embedded in a superconducting loop. Even without optimizing its design, this device shows extremely low flux noise, down to ∼10−5 Φ0Hz−1/2 (Φ0≃2×10−15 Wb is the flux quantum) and dissipation several orders of magnitude smaller than in conventional superconducting interferometers17,18,19. With optimization, the SQUIPT could significantly increase the sensitivity with which small magnetic moments are detected.
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Main
One typical SQUIPT fabricated with electron-beam lithography is shown in Fig. 1a. It consists of an aluminium (Al) superconducting loop interrupted by a copper (Cu) normal-metal wire in good electric contact with it. Furthermore, two Al electrodes are tunnel-coupled to the normal region to enable the device operation. A detailed view of the sample core (see Fig. 1b) shows the Cu region of length L≃1.5 μm and width ≃240 nm coupled to the tunnel probes and the superconducting loop. The SQUIPTs were implemented into two different designs (see Fig. 1c), namely, the A-type configuration, where the loop extends into an extra third lead, and the B-type configuration, which contains only two tunnel probes. The ring geometry enables us to change the phase difference across the normal-metal/superconductor boundaries through the application of an external magnetic field, which gives rise to a total flux Φ through the loop area. This modifies the DOS in the normal metal, and hence the transport through the tunnel junctions.
Insight into the interferometric nature of the SQUIPT can be gained by first analysing the theoretical prediction of its behaviour. Figure 2a shows the simplest implementation of the device in the A-type configuration, that is, that with just one junction tunnel-coupled to the normal metal. For simplicity, we suppose the tunnel probe (with resistance RT) to be placed in the middle of the wire, and to feed a constant electric current I through the circuit while the voltage drop V is recorded as a function of Φ. In the limit that the kinetic inductance of the superconducting loop is negligible, the magnetic flux fixes a phase difference φ=2πΦ/Φ0 across the normal metal, where Φ0=πℏ/e is the flux quantum, ℏ is the reduced Planck’s constant and e is the electron charge. Figure 2b shows the low-temperature quasiparticle current–voltage (I–V) characteristic of the SQUIPT calculated at a few selected values of Φ. The calculations were carried out for parameters similar to those of our structures20. Whereas for Φ=0, that is, when the minigap in the normal metal is maximized15,16, the characteristic resembles that of a superconductor–insulator–superconductor junction18, for Φ=Φ0/2 the characteristic corresponds to that of a normal-metal/insulator/superconductor contact, with the minigap suppressed15,16. The SQUIPT thus behaves as a flux-to-voltage transformer for which the response V(Φ) (and amplitude δ V) depends on the bias current I through the tunnel junction. The interferometer voltage modulation V(Φ) is shown in Fig. 2c for different values of I. In particular, V(Φ) is strongly dependent on the bias current, the latter determining the exact shape of the device response. Note the change of concavity of V(Φ), which occurs as the bias current exceeds the point where the I–V characteristics cross. One relevant figure of merit of the SQUIPT is represented by the flux-to-voltage transfer function, ∂ V/∂ Φ, which is shown in Fig. 2d. It turns out that ∂ V/∂ Φ is a non-monotonic function of the bias current, as well as its sign depending on the specific value of I.
Figure 3a shows the experimental low-temperature I–V characteristic of a device implemented in the A-type configuration. The curve resembles that of a typical superconducting tunnel junction, where the onset of large quasiparticle current is set by the energy gap (Δ0≃200 μeV in our samples). The absence of the peak in the experimental curves, as compared with the theoretical ones in Fig. 2b, could originate from broadening resulting from inelastic scattering or finite quasiparticle lifetime in the superconductor21. A deeper inspection reveals, however, that the characteristic is modulated by the presence of an applied magnetic field. The effect is clearly visible in Fig. 3b, which shows a detailed view of the curve at large bias voltage for some values of the applied flux up to Φ0/2. Such a modulation is of coherent nature, and stems from magnetic-field-induced control of the DOS in the normal metal. In addition to the quasiparticle current, a Josephson coupling is observed at the lowest temperatures, and manifests itself as a peak around zero bias in the I–V characteristic (see the inset of Fig. 3a). The supercurrent, which is expected to exist in proximized structures such as the present one12, obtains values as high as ≃17 pA at 53 mK. It is modulated by the applied flux with the same periodicity as for the quasiparticle current.
The full V(Φ) dependence for the same A-type sample at several values of the bias current is shown in Fig. 4a. As expected (see Fig. 2c), the modulation amplitude δ V is a non-monotonic function of I, and V(Φ) shows a change of concavity whenever the bias current exceeds the crossing points of the current–voltage characteristic (see Fig. 3b). In this sample, δ V obtains values as large as ∼7 μV at 1 nA. The corresponding transfer function is shown in Fig. 4b for a few bias currents. A resemblance to the theoretical prediction of Fig. 2c,d is obvious. In such a case, |∂ V/∂ Φ| as large as ≃30 μV/Φ0 is obtained at 1 nA. The maximum of |∂ V/∂ Φ| for the same SQUIPT is shown in Fig. 4c, and highlights the expected non-monotonic dependence on I.
Figure 4d and e show V(Φ) and the maximum of |∂ V/∂ Φ|, respectively, for a B-type SQUIPT. δ V obtains in this case values as high as ∼12 μV at 1 nA, and |∂ V/∂ Φ| is maximized at 0.6 nA where it reaches ≃60 μV/Φ0. We emphasize that these values are larger by almost a factor of two than those obtained in the A-type device. This is to be expected because in a B-type sample, V(Φ) is probed across two tunnel junctions in series. This doubles the SQUIPT response. The above results are roughly ∼50–60% of those predicted by our calculations (see Fig. 2), which can be ascribed either to the uncertainty in the precise determination of the device parameters20 or to non-ideal phase biasing of the interferometers15. In the limit of negligible geometric inductance of the loop (∼40 pH for our rings), a phase difference φ=2πΦ/Φ0 can be induced across the normal metal if the phase accumulated in the superconductor is much smaller than that accumulated in the wire, that is, if the ratio between their respective kinetic inductances is much smaller than unity. We estimate the kinetic inductance of the superconducting loop to be of the order of ∼150 pH, whereas that of the wire to be around ∼300–500 pH, so that the correction factor to the actual phase bias determined by such a ratio (∼0.3–0.5 for our devices) may prevent the full closing of the minigap, thus weakening the SQUIPT response.
The role of temperature (T) is shown in Fig. 5a, which shows V(Φ) at 1 nA for several increasing temperatures for a B-type sample. δ V initially monotonically decreases with increasing T up to ∼400 mK, then it starts to increase again and it is almost suppressed at 730 mK. The full temperature dependence of the maximum of |∂ V/∂ Φ| at 1 nA is shown in Fig. 5b for the same device, and reflects the above non-monotonic behaviour similarly to that observed for different bias currents (see Fig. 4c).
Compared with conventional d.c. superconducting quantum interference devices17,18,19 (SQUIDs), power dissipation (P) is markedly suppressed in the SQUIPT. In our devices we have P∼102 fW, which can be further reduced by simply increasing the resistance of the probing junctions. This power is four–five orders of magnitude smaller than that in conventional d.c. SQUIDs, which makes the SQUIPT ideal for applications where very low dissipation is required.
We shall finally comment on another figure of merit of the SQUIPT, namely, its noise-equivalent flux (NEF) or ‘flux sensitivity’, defined as NEF=〈VN2〉1/2/|∂ V/∂ Φ|δ ν1/2 (ref. 19), where VN is the voltage noise of the interferometer within the frequency band δ ν. In our experiment, we can provide an upper estimate for NEF, because it is believed to be limited mainly by the preamplifier noise. With a typical r.m.s. noise of ∼1.2 nV Hz−1/2 in our set-up, we estimate NEF≃2×10−5Φ0 Hz−1/2 at best (with the onset of 1/f noise roughly below ∼1 Hz), which should be substantially higher than the SQUIPT intrinsic NEF. Assuming that the noise of the interferometer is essentially of Johnson type, the intrinsic VN can be estimated by noting that in the range of experimental bias currents the device dynamic resistance is typically within the range ∼25–70 kΩ, leading to VN∼0.3–0.5 nV Hz−1/2 and NEF≃5–8 μΦ0 Hz−1/2 at 54 mK. We note that the preamplifier contribution to the noise can be made negligible by increasing |∂ V/∂ Φ|, that is, by optimizing the SQUIPT parameters (for instance, by choosing a superconducting material with a larger gap and by making a shorter normal-metal wire) and the phase bias as well. Our calculations show that by replacing niobium (Nb) as the superconductor (with Δ0≃1.5 meV), and by shortening L down to 150 nm, |∂ V/∂ Φ| as large as ∼2.5 mV/Φ0 could be achieved, yielding a preamplifier NEF≃4×10−7Φ0 Hz−1/2. The device intrinsic noise deserves however further investigation.
The SQUIPT has a number of features that make it attractive for a variety of applications: (1) only a simple d.c. read-out scheme is required, similarly to d.c. SQUIDs; (2) either current- or voltage-biased measurement can be conceived depending on the set-up requirements; (3) a large flexibility in the fabrication parameters and materials, such as semiconductors6,9, carbon nanotubes2,3,5 or graphene1 instead of normal metals, is allowed to optimize the response and the operating temperature (to this end superconducting V (ref. 22) or Nb are suitable candidates); (4) ultralow dissipation (∼1…100 fW), which makes it ideal for nanoscale applications; (5) ease of implementation in a series or parallel array (depending on the biasing mode) for enhanced output; and (6) ease of integration with superconducting refrigerators23 to actively tune the device working temperature. Finally, as far as specific applications24 are concerned, measurements of small magnetic systems25 (for instance, the magnetic flux induced by atomic spins as well as single-molecule nanomagnets), single-photon detection26, scanning microscopy as well as quantum metrology27 and nanoelectromechanical measurements28 with SQUIPT devices could be predicted. Our approach opens the way to magnetic-field detection based on ‘hybrid’ interferometers that take advantage of the flexibility intrinsic to proximity metals.
Methods
Fabrication details and experimental set-up.
The samples were fabricated at the Low Temperature Laboratory at Aalto University School of Science and Technology by standard three-angle shadow-mask evaporation of the metals through a conventional suspended resist mask in a single vacuum cycle. Initially, a bilayer poly(methyl methacrylate)/copolymer resist was spun on an oxidized Si wafer, onto which the structures were patterned using electron-beam lithography. In the electron-gun evaporator, the chip was first tilted to an angle of 25∘ with respect to the source, and approximately 27 nm of Al was evaporated to create the superconducting electrodes of the probe tunnel junctions. To form the tunnel barriers, the sample was exposed to 4.4 mbar of oxygen for five minutes, and consequently tilted to −25∘ for the deposition of 27 nm of Cu forming the normal-metal island. Immediately after this, the chip was tilted to the final angle of 9∘, and 60 nm of Al was deposited to form the superconducting loop and the transparent normal-metal/superconductor contacts. The magneto-electric characterization was carried out at NEST Istituto Nanoscienze-CNR by cooling the devices with a filtered 3He/4He dilution refrigerator down to ≃50 mK. Current and voltage were measured with room-temperature preamplifiers.
Theoretical model.
The considered system consists of a one-dimensional diffusive normal-metal wire of length L in good electric contact with two superconducting leads, which define a ring (see Fig. 2a). The contact with the superconductors enables superconducting correlations to be induced into the normal-metal region through the proximity effect11, which is responsible for the modification of the DOS in the wire13, as well as for the Josephson current to flow through the superconductor/normal-metal/superconductor structure12. The proximity effect in the normal-metal region of the SQUIPT can be described with the Usadel equations29, which can be written as12,29
where D is the diffusion constant and E is the energy relative to the chemical potential in the superconductors. θ and χ are, in general, complex scalar functions of position x and energy. For perfectly transmitting interfaces, the boundary conditions at the normal-metal/superconductor contacts (that is, x=±L/2, see Fig. 2a) reduce to θ(±L/2)=arctanh(Δ/E) and χ(±L/2)=±φ/2, where φ is the phase difference across the normal-metal/superconductor boundaries and Δ is the superconducting order parameter. For simplicity, we chose a step-function form for the order parameter, that is, constant in the superconductor and zero in the normal-metal region, although Δ is in principle position dependent and can be determined self-consistently12. The DOS in the normal-metal region normalized to the DOS at the Fermi level in the absence of the proximity effect is given by NN(x,E,φ)=Re{cosh[θ(x,E,φ)]}. From the numerical solution of equations (1), we get the DOS as a function of position and energy for any given φ. In particular, the DOS is an even function of energy, and has a minigap (Eg) for |E|≤Eg (ref. 13) with a magnitude that depends in general on the Thouless energy ETh=ℏD/L2, the characteristic energy scale for the normal region, and on φ. The minigap Eg is maximum for φ=0 and decreases with increasing φ, vanishing at φ=π (ref. 16; the behaviour is 2π-periodic in φ).
The quasiparticle current (Iqp) through the superconducting tunnel junction biased at voltage V (see Fig. 2a) can be calculated from30
where e is the electron charge, RT is the tunnel junction resistance, is the Bardeen–Cooper–Schrieffer-normalized DOS in the superconductor, Θ(z) is the Heaviside step function, f0(E)=(1+exp[E/(kBT)])−1 is the Fermi–Dirac distribution function at temperature T and kB is the Boltzmann constant. For any bias current (Ibias) imposed across the SQUIPT, the voltage response V(φ) is determined from the solution of the equation Ibias−Iqp(x,φ,T)=0. From this, we calculate the flux-to-voltage transfer function ∂ V/∂ φ.
Change history
10 June 2010
In the original version of this Letter published online, we had inadvertently neglected to cite some prior works that described a related device known as an Andreev interferometer. We apologize for this oversight.
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Acknowledgements
We gratefully acknowledge O. Astafiev, L. Faoro, R. Fazio, M. E. Gershenson, T. T. Heikkilä, L. B. Ioffe, V. Piazza, P. Pingue, F. Portier, H. Pothier, H. Rabani, F. Taddei and A. S. Vasenko for fruitful discussions. The work was partially supported by the INFM-CNR Seed project ‘Quantum-Dot Refrigeration: Accessing the μK Regime in Solid-State Nanosystems’, and by the NanoSciERA project ‘NanoFridge’.
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F.G. conceived and carried out the experiment, analysed the data, carried out the calculations and wrote the manuscript. M.M. took part in the early stage of measurements, contributed to the cryogenic set-up and to writing the manuscript. J.T.P. designed and fabricated the samples, and contributed to writing the manuscript. J.P.P. took part in the early stage of measurements, contributed to the cryogenic set-up, took part in the interpretation of the data and contributed to writing the manuscript. F.G. and J.P.P. discussed the results and implications and commented on the manuscript at all stages equally.
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Giazotto, F., Peltonen, J., Meschke, M. et al. Superconducting quantum interference proximity transistor. Nature Phys 6, 254–259 (2010). https://doi.org/10.1038/nphys1537
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DOI: https://doi.org/10.1038/nphys1537
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