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| Open AccessArbitrary engineering of spatial caustics with 3D-printed metasurfaces
Caustics, as a unique type of singularity in wave phenomena, occur in diverse physical systems. Here, the authors realize multi-dimensional customization of caustics with 3D-printed metasurfaces. This arbitrary caustic engineering is poised to bring new revolutions to many domains.
- Xiaoyan Zhou
- , Hongtao Wang
- & Cheng-Wei Qiu
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Article
| Open AccessMulti-site integrated optical addressing of trapped ions
A promising strategy for scaling trapped-ion-based quantum technologies is to use fully integrated optical waveguides to deliver light to numerous ions at multiple sites. Here, the authors. optically address three ions using on-chip waveguides to deliver three distinct wavelengths per ion, and perform Rabi flopping on each ion simultaneously.
- Joonhyuk Kwon
- , William J. Setzer
- & Hayden J. McGuinness
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Article
| Open AccessDelayed room temperature phosphorescence enabled by phosphines
Room-temperature phosphorescence usually occurs immediately after the removal of excitation. Here the authors achieve combined instant and delayed phosphorescence through introduction of phosphines into carbazole emitters.
- Guang Lu
- , Jing Tan
- & Hui Xu
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Article
| Open AccessPhotonic time-crystalline behaviour mediated by phonon squeezing in Ta2NiSe5
Photonic time crystal refers to a material whose dielectric properties oscillate in time. Here the authors theoretically show such behaviour in the excitonic insulator candidate Ta2NiSe5 under optical excitation and use it to explain the enhanced THz reflectivity recently observed in pump-probe experiments
- Marios H. Michael
- , Sheikh Rubaiat Ul Haque
- & Eugene Demler
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Article
| Open AccessDirect programming of confined surface phonon polariton resonators with the plasmonic phase-change material In3SbTe2
Tailored light-matter interaction can be achieved with surface phonon polaritons (SPhPs). Here, Conrads et al. employ the plasmonic phase-change material In3SbTe2 on the polar crystal SiC for direct programming of confined SPhP resonators and study their resonance modes via near-field microscopy.
- Lukas Conrads
- , Luis Schüler
- & Thomas Taubner
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Article
| Open AccessNeural étendue expander for ultra-wide-angle high-fidelity holographic display
All holographic displays and imaging techniques are fundamentally limited by the étendue supported by existing spatial light modulators. Here, the authors report on using artificial intelligence (AI) to learn an étendue expanding element that effectively increases étendue by two orders of magnitude.
- Ethan Tseng
- , Grace Kuo
- & Felix Heide
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Article
| Open AccessHigh-throughput quantum photonic devices emitting indistinguishable photons in the telecom C-band
An efficient way of realising a large number of telecom single-photon emitters for quantum communication is still missing. Here, the authors use a wide-field imaging technique for fast localization of single InAs/InP quantum dots, which are then integrated into circular Bragg grating cavities featuring high single-photon purity and indistinguishability.
- Paweł Holewa
- , Daniel A. Vajner
- & Elizaveta Semenova
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| Open AccessUltrastrong exciton-plasmon couplings in WS2 multilayers synthesized with a random multi-singular metasurface at room temperature
Here, the authors fabricate a metasurface with nanometre-sized plasmonic hotspots that interact coherently with WS2 excitons, achieving ultrastrong exciton-plasmon coupling.
- Tingting Wu
- , Chongwu Wang
- & Yu Luo
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Article
| Open AccessUltrafast photoluminescence and multiscale light amplification in nanoplasmonic cavity glass
This article presents a unique nanocomposite plasmonic-excitonic glass with extraordinary amplified optical properties: ultra-narrow photoluminescence (FWHM = 13 nm) and ultrashort photoluminescence lifetime (90 ps) at room temperature
- Piotr Piotrowski
- , Marta Buza
- & Dorota A. Pawlak
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Article
| Open AccessCorrelation-driven nonequilibrium exciton site transition in a WSe2/WS2 moiré supercell
Correlated insulator states of moire excitons in transition metal dichalcogenide heterostructures have attracted significant attention recently. Here the authors use time-resolved pump-probe spectroscopy to demonstrate the effects of non-equilibrium correlations of moire excitons in WSe2/WS2 heterobilayers.
- Jinjae Kim
- , Jiwon Park
- & Hyunyong Choi
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Article
| Open AccessAn optoacoustic field-programmable perceptron for recurrent neural networks
Optical recurrent neural networks present a unique challenge for photonic machine learning. Here, the authors experimentally show the first optoacoustic recurrent operator based on stimulated Brillouin scattering which may unlock a new class of optical neural networks with recurrent functionality.
- Steven Becker
- , Dirk Englund
- & Birgit Stiller
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Article
| Open AccessExtreme terahertz magnon multiplication induced by resonant magnetic pulse pairs
The authors demonstrate high-order terahertz nonlinear magnonics using two-dimensional coherent spectroscopy, revealing the emergence of seventh-order spin-wave mixing and sixth harmonic magnon generation within an antiferromagnetic orthoferrite.
- C. Huang
- , L. Luo
- & J. Wang
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| Open AccessRoom-temperature quantum emission from interface excitons in mixed-dimensional heterostructures
Interlayer excitons in 2D homo- and heterostructures have been intensively investigated due to their emerging optical properties. Here, the authors report the observation of interface excitons in 1D/2D carbon nanotube/WSe2 heterostructures, showing evidence of photon antibunching at room temperature.
- N. Fang
- , Y. R. Chang
- & Y. K. Kato
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Article
| Open AccessGiant Faraday rotation in atomically thin semiconductors
Here, the authors perform Faraday rotation spectroscopy around the excitonic transitions in hBN-encapsulated WSe2 and MoSe2 monolayers, and interlayer excitons in MoS2 bilayers. They measure a large Verdet constant - 1.9 × 107 deg T−¹cm−¹ for monolayers, and attribute it to the giant oscillator strength and high g-factor of the excitons.
- Benjamin Carey
- , Nils Kolja Wessling
- & Ashish Arora
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Article
| Open AccessObservation of spatiotemporal optical vortices enabled by symmetry-breaking slanted nanograting
A microscale platform composed of a slanted nanograting is experimentally demonstrated to efficiently generate spatiotemporal optical vortex. This approach paves the way towards an integrated system for ultrafast pulse shaping.
- Pengcheng Huo
- , Wei Chen
- & Ting Xu
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Article
| Open AccessFast joint parity measurement via collective interactions induced by stimulated emission
Parity detection is essential in quantum error correction. Here, authors propose a reliable joint parity measurement (JPM) scheme inspired by stimulated emission and experimentally implement the weight-2(4) JPM scheme in a tunable coupling superconducting circuit, which shows comparable performance to the standard CNOT-gate based scheme.
- Sainan Huai
- , Kunliang Bu
- & Yicong Zheng
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Article
| Open AccessIntercavity polariton slows down dynamics in strongly coupled cavities
Band engineering in optics allows the design of unconventional forms of light with potential optoelectronic applications. Here, the authors realize slow-light intercavity polaritons in an array of coupled cavities, the photonic architecture enables the spatial segregation of photons and excitons
- Yesenia A. García Jomaso
- , Brenda Vargas
- & Giuseppe Pirruccio
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Article
| Open AccessLarge area single crystal gold of single nanometer thickness for nanophotonics
2D metallic single crystals are sought after for nanophotonic applications, but their synthesis remains challenging. Here, the authors report an atomic level precision etching method to fabricate large-area crystalline gold flakes with nanometre thickness, showing enhanced plasmonic and nonlinear optical properties.
- Chenxinyu Pan
- , Yuanbiao Tong
- & Pan Wang
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Article
| Open AccessDynamic switching from coherent perfect absorption to parametric amplification in a nonlinear spoof plasmonic waveguide
The authors propose a nonlinear spoof plasmonic waveguide to realize coherent perfect absorption and parametric amplification at the same frequency, which opens a new route to actively modulate the electromagnetic waves with giant amplification-to-absorption contrast.
- Wen Yi Cui
- , Jingjing Zhang
- & Tie Jun Cui
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Article
| Open AccessHyperbolic metamaterial empowered controllable photonic Weyl nodal line semimetals
One-dimensional photonic crystals provide a platform to modulate Weyl quasiparticles with properties of bound states in the continuum both dynamically (transition and rotation) and topologically (singularities in bilateral drumhead surface states).
- Shengyu Hu
- , Zhiwei Guo
- & Hong Chen
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| Open AccessEfficient excitation and control of integrated photonic circuits with virtual critical coupling
The authors achieve enhanced cavity loading using complex-frequency excitations that can tailor on-demand the effective coupling rate in a microring resonator by precisely controlling the temporal evolution of the incident pulses.
- Jakob Hinney
- , Seunghwi Kim
- & Michal Lipson
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| Open AccessRaman time-delay in attosecond transient absorption of strong-field created krypton vacancy
The advent of isolated attosecond XUV pulse sources marks a new era in attosecond science, pivotal for the investigation of core electron dynamics. Here the authors discover that the coherent Raman coupling between the cation states leads to extra timedelay between different transition channels by applying the attosecond transient absorption spectroscopy on the investigation of complex dynamics of strong field ionization of Krypton.
- Li Wang
- , Guangru Bai
- & Zengxiu Zhao
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Article
| Open AccessDemonstration of hypergraph-state quantum information processing
Usual multiqubit entangled states can be described using the graph formalism, where each edge connects only two qubits. Here, instead, the authors use a reprogrammable silicon photonics chip to showcase preparation, verification and processing of arbitrary four-qubit hypergraph states, where hyperedges describe entanglement within a subset of many qubits.
- Jieshan Huang
- , Xudong Li
- & Jianwei Wang
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Article
| Open AccessDefect-induced helicity dependent terahertz emission in Dirac semimetal PtTe2 thin films
Defect engineering of topological materials provides an avenue for the controllable manipulation of optoelectronic properties. Here, the authors introduce a defect gradient into a Dirac semimetal to control the Berry curvature dipole-driven THz emission in the material.
- Zhongqiang Chen
- , Hongsong Qiu
- & Xuefeng Wang
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Article
| Open AccessTunable anisotropic van der Waals films of 2M-WS2 for plasmon canalization
Anisotropic light-matter excitations in van der Waals materials are expected to have an impact on nanophotonics applications. Here, the authors report the observation of canalized in-plane mid-infrared plasmons in the semimetallic phase of WS2 and demonstrate their electrical tunability via ion intercalation.
- Qiaoxia Xing
- , Jiasheng Zhang
- & Hugen Yan
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Article
| Open AccessUniversal control of a bosonic mode via drive-activated native cubic interactions
Manipulating quantum information encoded in a bosonic mode requires sizeable and controllable nonlinearities, but superconducting devices’ strong nonlinearities are normally static. Here, the authors use a SNAIL to suppress static nonlinearities and use drive-dependent ones to reach universal control of a bosonic mode.
- Axel M. Eriksson
- , Théo Sépulcre
- & Simone Gasparinetti
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Article
| Open AccessHigh performance artificial visual perception and recognition with a plasmon-enhanced 2D material neural network
Here, the authors demonstrate a low-power neuromorphic visual architecture based on a plasmon-enhanced 2D semiconductor phototransistor array, showing high-speed sensing, preprocessing and image recognition functionalities.
- Tian Zhang
- , Xin Guo
- & Linjun Li
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Article
| Open AccessPoincaré sphere trajectory encoding metasurfaces based on generalized Malus’ law
Polarization serves as an excellent information encoding carrier. Here, authors expand the metasurface encoding dimensionality of polarization information by engineering the Poincaré Sphere trajectory with generalized Malus’ law, unveiling new opportunities for advanced polarization optics.
- Zi-Lan Deng
- , Meng-Xia Hu
- & Andrea Alù
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Article
| Open AccessHermitian and non-Hermitian topology from photon-mediated interactions
Topological properties of a photonic environment are crucial to engineer robust photon-mediated interactions between quantum emitters. Here, the authors find general theorems on the topology of photon-mediated interactions, unveiling the phenomena of topological preservation and reversal.
- Federico Roccati
- , Miguel Bello
- & Angelo Carollo
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| Open AccessCavity-coupled telecom atomic source in silicon
T centers in silicon are promising candidates for quantum applications yet suffer from weak optical transitions. Here, by integrating with a silicon nanocavity, the authors demonstrate an enhancement of the photon emission rate for a single T center.
- Adam Johnston
- , Ulises Felix-Rendon
- & Songtao Chen
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Article
| Open AccessUltra-compact exciton polariton modulator based on van der Waals semiconductors
Miniaturized and efficient optical modulators are desired for data transmission, processing and communication. Here, the authors report the fabrication of exciton-polariton Mach–Zehnder modulators based on thin WS2 waveguides with a footprint of ~30 μm², modulation ratio up to −6.20 dB and nanosecond response times.
- Seong Won Lee
- , Jong Seok Lee
- & Su-Hyun Gong
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Article
| Open AccessTime-of-flight detection of terahertz phonon-polariton
Polaritons, light-matter hybridized quasiparticles, are the fundamental excitation of strong coupling systems and are widely applicable in information technologies. Here the authors applied the concept of time-of-flight measurement in terahertz induced second harmonic generation experiments in various systems to comprehensively study the dispersion relation of phonon-polaritons and reveal potential spin-lattice couplings.
- Tianchuang Luo
- , Batyr Ilyas
- & Nuh Gedik
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Article
| Open AccessRoom-temperature strong coupling in a single-photon emitter-metasurface system
Interfacing single-photon emitters (SPEs) with high-finesse cavities can prevent decoherence processes, especially at elevated temperature, but its implementation remains challenging. Here, the authors report room-temperature strong coupling of SPEs in hexagonal boron nitride with a dielectric cavity based on bound states in the continuum, showing a Rabi splitting of ~ 4 meV.
- T. Thu Ha Do
- , Milad Nonahal
- & Son Tung Ha
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Article
| Open AccessBroadband angular spectrum differentiation using dielectric metasurfaces
Metasurfaces processing incoming images have been proposed in the context of real space operations. Here, the authors demonstrate mathematical operations, such as differentiation, on the angular spectrum of an image using metasurfaces, which can be used to enhance spectral features of an image.
- Ming Deng
- , Michele Cotrufo
- & Lin Chen
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| Open AccessRetinal photoisomerization versus counterion protonation in light and dark-adapted bacteriorhodopsin and its primary photoproduct
Malakar et al. investigate the photochemical dynamics in the isomerization of bacteriorhodopsin light and dark-adapted forms and in the first photocycle intermediate, K. The results prompt a reevaluation of the counter ion model, revealing that a different protonation then that shown in the classic quadrupole so far considered must be employed to account for the experimental data.
- Partha Malakar
- , Samira Gholami
- & Sanford Ruhman
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| Open AccessBerkSEL: A scale-invariant laser beyond the Schawlow-Townes two-mirror strategy
I argue that a surface emitting laser that remains single mode irrespective of its size, a scale-invariant laser, should of necessity also waste light at the edge. This is a fundamental departure from the Schawlow-Townes two-mirror strategy that keeps light away from mirrors and edges to preserve gain and minimize loss. The strategy was implemented in the recent discovery of the Berkeley Surface Emitting Laser (BerkSEL).
- Boubacar Kanté
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Article
| Open AccessSpectral-temporal-spatial customization via modulating multimodal nonlinear pulse propagation
The authors introduce a method for modulating the multimodal nonlinear pulse propagation in fibers by controlled bending, achieving a tunable broadband high-peak-power femtosecond light source that could empower nonlinear imaging and spectroscopy.
- Tong Qiu
- , Honghao Cao
- & Sixian You
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Article
| Open AccessWandering principal optical axes in van der Waals triclinic materials
Principal optical axes define light-matter interactions in crystals and they are usually assumed to be stationary. Here, the authors report the observation of wavelength-dependent principal optical axes in ternary van der Waals crystals (ReS2 and ReSe2), leading to wavelength-switchable propagation directions of their waveguide modes.
- Georgy A. Ermolaev
- , Kirill V. Voronin
- & Kostya S. Novoselov
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Article
| Open AccessOptically addressable spin defects coupled to bound states in the continuum metasurfaces
Previous research reported enhanced emission from spin defects in hBN by coupling to optical resonators; however, this approach has limited scalability. Here the authors use a monolithic metasurface featuring quasi bound states fabricated from hBN to enhance photoemission and optical spin-readout efficiency of defects in the same material.
- Luca Sortino
- , Angus Gale
- & Andreas Tittl
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Article
| Open AccessNon-Hermitian non-equipartition theory for trapped particles
The authors propose a generalization of the equipartition theorem of thermal physics to account for non-Hermitian trapping forces, relevant for the problems in non-equilibrium open systems and advanced nanotechnology.
- Xiao Li
- , Yongyin Cao
- & Jack Ng
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Article
| Open AccessProbing molecules in gas cells of subwavelength thickness with high frequency resolution
Using gas cells for spectroscopic studies opens possibility for miniaturized platforms that can be integrated with other optical components. Here the authors demonstrate molecular rovibrational spectroscopy by confining molecules in a cell of subwavelength thickness.
- Guadalupe Garcia Arellano
- , Joao Carlos de Aquino Carvalho
- & Athanasios Laliotis
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Article
| Open AccessCoherent control of enhanced second-harmonic generation in a plasmonic nanocircuit using a transition metal dichalcogenide monolayer
Here, the authors integrate monolayer MoSe2 with a plasmonic nanocircuit and demonstrate the coherent selective routing of the enhanced nonlinear optical signal emitted by the 2D semiconductor, with routing extinction ratios up to 14.86 dB.
- Pei-Yuan Wu
- , Wei-Qing Lee
- & Chen-Bin Huang
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Article
| Open AccessElectron/infrared-phonon coupling in ABC trilayer graphene
Via Raman and infrared spectroscopy measurements, X. Zan et al. find that rhombohedral ABC trilayer graphene has stronger electron/infrared-phonon coupling than Bernal ABA trilayer graphene.
- Xiaozhou Zan
- , Xiangdong Guo
- & Guangyu Zhang
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Article
| Open AccessMode-multiplexing deep-strong light-matter coupling
The authors show an original approach to achieve strong light-matter interaction harnessing the coupling between plasmonic resonators and the Landau resonances of an underlying quantum well, demonstrating remarkably high coupling strengths.
- Joshua Mornhinweg
- , Laura Katharina Diebel
- & Christoph Lange
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Article
| Open AccessLight-induced switching between singlet and triplet superconducting states
S. Gassner et al. propose using light pulses to drive a centrosymmetric s-wave superconductor with strong spin-orbit coupling into a metastable triplet p-wave superconductor with non-trivial topology. The two superconducting orders must be closely competing in equilibrium and the light pulse must break a generalized, dynamic form of inversion symmetry.
- Steven Gassner
- , Clara S. Weber
- & Martin Claassen
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Article
| Open AccessReconfigurable perovskite X-ray detector for intelligent imaging
In-sensor computing requires detectors with polarity reconfigurability and linear responsivity. Pang et al. report a CsPbBr3 perovskite single crystal X-ray detector for edge extraction imaging with a data compression ratio of 46.4% and classification task with an accuracy of 100%.
- Jincong Pang
- , Haodi Wu
- & Guangda Niu
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Article
| Open AccessEnergy transfer driven brightening of MoS2 by ultrafast polariton relaxation in microcavity MoS2/hBN/WS2 heterostructures
Here, the authors design a microcavity-confined 2D heterojunction to realize the strong coupling among donor exciton, acceptor exciton, and cavity photon mode, leading to an unconventional energy transfer via polariton relaxation with an enhancement factor of ~440.
- Zehua Hu
- , Tanjung Krisnanda
- & Qihua Xiong
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Article
| Open AccessStrong interactions between solitons and background light in Brillouin-Kerr microcombs
Here the authors demonstrate a strong interaction between the generated solitons and background light in a Brillouin-Kerr microcomb system. Based on this unique physical mechanism, they achieve a monostable single soliton microcomb and a turnkey single-soliton microcomb without employing any optical/electrical control or feedback.
- Menghua Zhang
- , Shulin Ding
- & Xiaoshun Jiang
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Article
| Open AccessNonlinear spin-orbit coupling in optical thin films
Spin-orbit interaction, and the associated phenomena, is commonly observed in crystalline structure pumped with circularly polarised beam. Here, the authors showed that this is not the case, and used nonlinear thin film to produce vortex beams of second-harmonic light.
- Domenico de Ceglia
- , Laure Coudrat
- & Costantino De Angelis
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